Bilayer splitting and c-axis coupling in bilayer manganites showing colossal magnetoresistance

C. Jozwiak, J. Graf, S. Y. Zhou, A. Bostwick, Eli Rotenberg, H. Zheng, J. F. Mitchell, A. Lanzara

Published 2008-06-12, updated 2009-12-23Version 2

By performing angle-resolved photoemission spectroscopy of the bilayer colossal magnetoresistive (CMR) manganite, $La_{2-2x}Sr_{1+2x}Mn_{2}O_{7}$, we provide the complete mapping of the Fermi level spectral weight topology. Clear and unambiguous bilayer splitting of the in-plane 3d$_{x^2-y^2}$ band, mapped throughout the Brillouin zone, and the full mapping of the 3d$_{3z^2-r^2}$ band are reported. Peculiar doping and temperature dependencies of these bands imply that as transition from the ferromagnetic metallic phase approaches, either as a function of doping or temperature, coherence along the c-axis between planes within the bilayer is lost, resulting in reduced interplane coupling. These results suggest that interplane coupling plays a large role in the CMR transition.