{ "id": "1203.3905", "version": "v1", "published": "2012-03-17T23:23:58.000Z", "updated": "2012-03-17T23:23:58.000Z", "title": "Driven Brownian coagulation of polymers", "authors": [ "P. L. Krapivsky", "Colm Connaughton" ], "comment": "14 pages and 12 figures", "categories": [ "cond-mat.stat-mech" ], "abstract": "We present an analysis of the mean-field kinetics of Brownian coagulation of droplets and polymers driven by input of monomers which aims to characterize the long time behavior of the cluster size distribution as a function of the inverse fractal dimension, $a$, of the aggregates. We find that two types of long time behavior are possible. For $0\\leq a < 1/2$ the size distribution reaches a stationary state with a power law distribution of cluster sizes having exponent 3/2. The amplitude of this stationary state is determined exactly as a function of $a$. For $1/2 < a \\leq 1$, the cluster size distribution never reaches a stationary state. Instead a bimodal distribution is formed in which a narrow population of small clusters near the monomer scale is separated by a gap (where the cluster size distribution is effectively zero) from a population of large clusters which continue to grow for all time by absorbing small clusters. The marginal case, $a=1/2$, is difficult to analyze definitively, but we argue that the cluster size distribution becomes stationary and there is a logarithmic correction to the algebraic tail.", "revisions": [ { "version": "v1", "updated": "2012-03-17T23:23:58.000Z" } ], "analyses": { "subjects": [ "36.40.Mr", "36.20.Hb", "36.20.Ey", "31.15.X-" ], "keywords": [ "driven brownian coagulation", "cluster size distribution", "stationary state", "long time behavior", "small clusters" ], "tags": [ "journal article" ], "publication": { "doi": "10.1063/1.4718833", "journal": "Journal of Chemical Physics", "year": 2012, "month": "May", "volume": 136, "number": 20, "pages": 4901 }, "note": { "typesetting": "TeX", "pages": 14, "language": "en", "license": "arXiv", "status": "editable", "adsabs": "2012JChPh.136t4901K" } } }